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Two modifications for the basic Barcelona model (BBM) are present. One is the replacement of the net stress by the average skeleton stress in unsaturated soil modeling, and the other is the adoption of an expression for the load-collapse (LC) yield surface that can match flexibly the normal compression lines at different suctions. The predictions of the modified BBM for the controlled-suction triaxial test on the unsaturated compacted clay are presented and compared with the experimental results. A good agreement between the predicted and experimental results demonstrates the reasonability of the modified BBM. On this basis, the coupled processes of groundwater flow and soil deformation in a homogeneous soil slope under a long heavy rainfall are simulated with the proposed elasto-plastic model. The numerical results reveal that the failure of a slope under rainfall infiltration is due to both the reduction of soil suction and the significant rise in groundwater table. The evolution of the displacements is greatly related to the change of suction. The maximum collapse deformation happens near the surface of slope where infiltrated rainwater can quickly reach. The results may provide a helpful reference for hazard assessment and control of rainfall-induced landslides.