Hydrothermal Synthesis of Nanostructural La_xBi_(2-x)Se_yTe_(3-y) Powders

来源 :Journal of Rare Earths | 被引量 : 0次 | 上传用户:phenix519
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Nanostructural monophase La_xBi_ 2-xSe_yTe_ 3-y alloy was synthesized with a hydrothermal route using BiCl_3, LaCl_3, selenium and tellurium powders as the precursors, NaOH and disodium ethylenediaminetetraacetiate (EDTA) as the additives. The hydrothermally synthesized powders have a petal-like morphology self-structured by the parallel side-by-side arrangement of the nano-scales. It is found that an alkaline additive is necessary for the synthesis of a monophase Bi_2Te_3 based alloy. EDTA acts as a soft template for the lateral growth of the nano-scales and the self-constitution of the petal-like structure. It is found that the synthesis reaction can be however hindered by excessive EDTA. Nanostructural monophase La_xBi_2-xSe_yTe_3-y alloy was synthesized with a hydrothermal route using BiCl_3, LaCl_3, selenium and tellurium powders as the precursors, NaOH and disodium ethylenediaminetetraacetiate (EDTA) as the additives. The hydrothermally synthesized powders have a petal-like morphology self-structured by the parallel side-by-side arrangement of the nano-scales. It is found that an an alkaline additive is necessary for the synthesis of a monophase Bi 2 Te 3 based alloy. EDTA acts as a soft template for the lateral growth of the nano -scales and the self-constitution of the petal-like structure. It is found that the synthesis reaction can be but hindered by excessive EDTA.
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