In this study, TiO2 nanoforest films consisting of nanotubes have been synthesized by a simple hydrothermal method and a subsequent sintering technique. The hydrothermal reaction time is important for the controlling of the nanotube diameter and the specific surface area of holistic TiO2 films. When the hydrothermal process reaction time is up to 8 hours, the diameter of the nanotube is about 10 nm, and the specific surface area of TiO2 nanoforest films reaches the maximum. CdS nanoparticles are synthesized on TiO2 nanoforest films by the successive ionic layer adsorption and reaction (SILAR) technique. The transmission electron microscope (TEM) and energy dispersive x-ray spectroscopy (EDX) mapping results verify that TiO2/CdS heterostructures are realized. A significant red-shift of the absorption edge from 380 nm to 540 nm can be observed after the pure TiO2 film is sensitized by CdS nanoparticles. Under irradiation of light, the current density of the optimal TiO2/CdS photoanode is 2.30 mA·cm?2 at 0 V relative to the saturated calomel electrode (SCE), which is 6 times stronger than that of the pure TiO2 photoanode. This study suggests that the TiO2 nanoforest consisting of interlinked pony-size nanotubes is a promising nanostructure for photoelectrochemical.