Crystal structure and phase transition of 2-methoxyanilinium perchlorate-18-crown-6

来源 :Chinese Chemical Letters | 被引量 : 0次 | 上传用户:hj0411
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A new phase transition compound,2-methoxyanilinium perchlorate-18-crown-6(1) {(oCH3OC6H4NH3)+(18-crown-6) ClO4 },has been synthesized and separated as crystals.Differential scanning calorimetry(DSC) measurements show a pair of sharp peaks at 225 K(heating) and 210 K(cooling),indicating the phase transition is first-order.Dielectric anomalies observed at 225 K(heating)and 210 K(cooling) further confirm the phase transition.The crystal structures determined at 298 K and123 K are both triclinic in P 1.The most distinct difference between room-temperature and lowtemperature structures is the order–disorder transition of the host 18-crown-6 molecule,which is the driving force of the phase transition. A new phase transition compound, 2-methoxyanilinium perchlorate-18-crown-6 (1) {(oCH3OC6H4NH3) + (18- crown- 6) ClO4}, has been synthesized and separated as crystals. Differential scanning calorimetry A pair of sharp peaks at 225 K (heating) and 210 K (cooling), indicating the phase transition is first-order. Electricomalomalomal observed at 225 K (heating) and 210 K structures determined at 298 K and 123 K are both triclinic in P 1. The most distinct difference between room-temperature and lowtemperature structures is the order-disorder transition of the host 18-crown-6 molecule, which is the driving force of the phase transition .
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