Synthesis and Supramolecular Structure of Chloro(1,10-phenanthroline)copper(I) Hexahydrate

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The title compound, C24H28ClCuN4O6 (Mr = 567.49), has been prepared and its crystal structure has been determined by X-ray diffraction method. The crystal belongs to mono- clinic, space group C2/c with a = 23.1905(14), b = 30.1877(12), c = 7.4881(3) ?, β = 97.631(2)o, V = 5195.8(4) ?3, Z = 8, Dc = 1.451 g/cm3, μ = 0.989 mm–1, F(000) = 2352, S = 1.030, R = 0.0694, wR = 0.2120 (I > 2σ(I)), R = 0.0950 and wR = 0.2322 (all data). The crystal consists of the Cu(I) complex and lattice water molecules. The Cu(I) atom is coordinated by two phenanthroline (phen) molecules and one chlorine anion with a distorted trigonal dipyramidal coordination geometry. By the aid of aromatic π-π stacking, the Cu(I) complex molecules form two-dimensional supramo- lecular layers. Lattice water molecules locate between the adjacent layers to form a three-dimen- sional sandwich-like supramolecular structure. The title compound, C24H28ClCuN4O6 (Mr = 567.49), has been prepared and its crystal structure has been determined by X-ray diffraction method. The crystal belongs to mono- clinic, space group C2 / c with a = 23.1905 (14), b Β = 97.631 (2) o, V = 5195.8 (4)? 3, Z = 8, Dc = 1.451 g / cm3, μ = 0.989 mm-1, (000) = 2352, S = 1.030, R = 0.0694, wR = 0.2120 (I> 2σ (I)), R = 0.0950 and wR = 0.2322 (all data). The crystal consists of the Cu (I) complex and lattice water molecules. The Cu (I) atom is coordinated by two phenanthroline (phen) molecules and one chlorine anion with a distorted trigonal dipyramidal coordination geometry. By the aid of aromatic π-π stacking, the Cu (I) dimensional supramo-lecular layers. Lattice water molecules locate between the adjacent layers to form a three-dimen- sional sandwich-like supramolecular structure.
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