Facile Synthesis of Nanocrystal Tin Oxide Hollow Microspheres by Microwave-Assisted Spray Pyrolysis

来源 :Journal of Materials Science & Technology | 被引量 : 0次 | 上传用户:hnbc2008
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Tin oxide(SnO_2) hollow microspheres with narrow size distribution were prepared by a facile one-pot microwave-assisted spray pyrolysis method. The effect of temperature on microstructural and optical properties was investigated by X-ray diffraction(XRD), scanning electron microscope(SEM), high resolution transmission electron microscope(HRTEM), and UV-Vis spectrophotometer(UV-Vis), respectively.The SnO_2 particles obtained at and above 700?C are tetragonal rutile structure with high purity and smooth surface morphology, which consist of well-interconnected SnO_2 nanocrystallines and the shell thickness was about 26 nm. UV-Vis absorption values were quite low in visible light region and high in ultraviolet region, indicating the possible utilization for optical purpose of the as-prepared SnO_2. The band gaps were 3.88 and 4.07 e V for SnO_2 synthesized at 700 and 800?C, respectively. As compared to traditional electrical heating or flame modes, microwave heating introduced here demonstrates a highefficiency, environmentally benign, and time-and energy-saving technology to synthesize advanced powders. Tin oxide (SnO 2) hollow microspheres with narrow size distribution were prepared by a facile one-pot microwave-assisted spray pyrolysis method. The effect of temperature on microstructural and optical properties was investigated by X-ray diffraction (XRD) SEM), high resolution transmission electron microscope (HRTEM), and UV-Vis spectrophotometer (UV-Vis), respectively.The SnO 2 particles were obtained at 700 C C and tetragonal rutile structure with high purity and smooth surface morphology, which consist of Well-interconnected SnO 2 nanocrystallines and the shell thickness was about 26 nm. UV-Vis absorption values ​​were quite low in visible light region and high in ultraviolet region, indicating the possible utilization for optical purpose of the as-prepared SnO 2. The band gaps were 3.88 and 4.07 e V for SnO 2 synthesized at 700 and 800? C, respectively. As compared to traditional electrical heating or flame modes, microwave heating introduced here demonst rates a highefficiency, environmentally benign, and time-and energy-saving technology to synthesize advanced powders.
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