A facile synthesis of ω-aminoalkyl ammonium hydrogen phosphates

来源 :Chinese Chemical Letters | 被引量 : 0次 | 上传用户:asdfghjkd
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A series of v-aminoalkyl ammonium hydrogen phosphates were synthesized through a simple and efficient three-step method.The starting materials,v-aminoalkyl alcohols(AC-n,with carbon number n = 3,4,5,6),were amino-protected with 9fluorenylmethyl chloroformate(Fmoc-Cl),followed by phosphorylation with POCl 3 and deprotection in piperidine/DMF.The structures of each intermediate and final product were confirmed by 1 H NMR,FTIR and mass spectrum.The yield of each step was about 77-92%,with a total yield higher than 56%.This new method was superior in low-cost raw materials,mild reaction temperatures(0-25 8C) and easy purification methods. A series of v-aminoalkyl ammonium hydrogen phosphates were synthesized through a simple and efficient three-step method. The starting materials, v-aminoalkyl alcohols (AC-n, with carbon number n = 3,4,5,6) -protected with 9fluorenylmethyl chloroformate (Fmoc-Cl), followed by phosphorylation with POCl3 and deprotection in piperidine / DMF. The structures of each intermediate and final product were confirmed by1H NMR, FTIR and mass spectra. The yield of each step was about 77-92%, with a total yield higher than 56%. This new method was superior in low-cost raw materials, mild reaction temperatures (0-25 8C) and easy purification methods.
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